TA1 P-Ti/AA6061 composite plate was produced by oxidizing the surface of the titanium plate and adopting a cold roll bonding process. The results revealed that the oxide film (Ti₆O) prepared on the surface of TA1 pure titanium was easy to crack during the cold roll bonding, thereby promoting the formation of an effective mechanical interlock at the interface, which can effectively reduce the minimum reduction rate of the composite plates produced by cold rolling of titanium and aluminium plates. Moreover, the composite plate subjected to oxidation treatment exhibited high shear strength, particularly at a 43% reduction rate, achieving a commendable value of 117 MPa. Based on oxidation treatment and different reduction rates, the annealed composite plates at temperatures of 400, 450, and 500 °C displayed favorable resistance to interface delamination, highlighting their remarkable strength-plasticity compatibility as evidenced by a maximum elongation of 31.845%.